The battle between Labour incumbent Mr Khan and his Tory challenger Ms Hall is expected to be closer than expected. The first results on the mayoralty may come in around midday, with speculation that by around 1.30pm it might be clear who will emerge as the winner.
It comes as results of several other mayoral, council, and police and crime commissioner elections will also be announced on Saturday, after a bruising day of election results for Rishi Sunak, when the Conservatives suffered a net loss of 371 seats, and lost control of 10 councils.
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